Faculty Profiles - SHINOKUBO, Hiroshi

Papers - SHINOKUBO, Hiroshi

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Diazachlorin and diazabacteriochlorin for one- and two-photon photodynamic therapy. Reviewed

Longevial Jean-Francois, Yamaji Ayaka, Aggad Dina, Kim Gakhyun, Chia Wen Xi, Nishimura Tsubasa, Miyake Yoshihiro, Clement Sebastien, Oh Juwon, Daurat Morgane, Nguyen Christophe, Kim Dongho, Gary-Bobo Magali, Richeter Sebastien, Shinokubo Hiroshi

Chemical communications (Cambridge, England) Vol. 54 ( 98 ) page： 13829 - 13832 2018.12

Theoretical Study on Open-Shell Singlet Character and Second Hyperpolarizabilities in Cofacial π-Stacked Dimers Composed of Weak Open-Shell Antiaromatic Porphyrins Reviewed

Fujiyoshi Jun-ya, Tonami Takayoshi, Yamane Masaki, Okada Kenji, Kishi Ryohei, Muhammad Shabbir, Al-Sehemi Abdullah G, Nozawa Ryo, Shinokubo Hiroshi, Nakano Masayoshi

ChemPhysChem Vol. 19 ( 21 ) page： 2863 - 2871 2018.11

X-Shaped Cyclobutane-Linked Tetraporphyrins through a Thermal [2+2] Cycloaddition of Etheno-Fused Diporphyrins Reviewed

Nagai Tomohiro, Takiguchi Asahi, Ueda Masayuki, Oda Kazuma, Hiroto Satoru, Shinokubo Hiroshi

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY Vol. 140 ( 27 ) page： 8392-8395 2018.7

Azabuckybowl-Based Molecular Tweezers as C-60 and C-70 Receptors Reviewed

Takeda Motoki, Hiroto Satoru, Yokoi Hiroki, Lee Sangsu, Kim Dongho, Shinokubo Hiroshi

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY Vol. 140 ( 20 ) page： 6336-6342 2018.5

The reductive aromatization of naphthalene diimide: a versatile platform for 2,7-diazapyrenes Reviewed

Nakazato Takumi, Kamatsuka Takuto, Inoue Junichi, Sakurai Tsuneaki, Seki Shu, Shinokubo Hiroshi, Miyake Yoshihiro

CHEMICAL COMMUNICATIONS Vol. 54 ( 41 ) page： 5177-5180 2018.5

Reversible sigma-Bond Formation in Bowl-Shaped pi-Radical Cations: The Effects of Curved and Planar Structures Reviewed

Yokoi Hiroki, Hiroto Satoru, Shinokubo Hiroshi

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY Vol. 140 ( 13 ) page： 4649-4655 2018.4

Figuration of bowl-shaped pi-conjugated molecules: properties and functions Invited Reviewed

Saito Masaichi, Shinokubo Hiroshi, Sakurai Hidehiro

MATERIALS CHEMISTRY FRONTIERS Vol. 2 ( 4 ) page： 635 - 661 2018.4

Benzonorcorrole Ni-II Complexes: Enhancement of Paratropic Ring Current and Singlet Diradical Character by Benzo-Fusion Reviewed

Yoshida Takuya, Takahashi Kohtaro, Ide Yuki, Kishi Ryohei, Fujiyoshi Jun-ya, Lee Sangsu, Hiraoka Yuya, Kim Dongho, Nakano Masayoshi, Ikeue Takahisa, Yamada Hiroko, Shinokubo Hiroshi

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION Vol. 57 ( 8 ) page： 2209-2213 2018.2

Supramolecular assemblies of a nitrogen-embedded buckybowl dimer with C-60 Reviewed

Yokoi Hiroki, Hiroto Satoru, Sakamaki Daisuke, Seki Shu, Shinokubo Hiroshi

CHEMICAL SCIENCE Vol. 9 ( 4 ) page： 819-824 2018.1

Synthesis and Photodynamics of Tetragermatetrathia[8]circulene Reviewed

Akahori Shuhei, Sakai Hayato, Hasobe Taku, Shinokubo Hiroshi, Miyake Yoshihiro

ORGANIC LETTERS Vol. 20 ( 1 ) page： 304-307 2018.1

Nickel (II) pyrrocorphin: Enhanced binding ability in a highly reduced porphyrin complex. Reviewed

Ide Y, Kuwahara T, Takeshita S, Fujishiro R, Suzuki M, Mori S, Shinokubo H, Nakamura M, Yoshino K, Ikeue T

Journal of inorganic biochemistry Vol. 178 page： 115 - 124 2018.1

Synthesis of Heteroatom-Containing Curved pi-Conjugated Molecules Reviewed

Hiroto Satoru, Shinokubo Hiroshi

JOURNAL OF SYNTHETIC ORGANIC CHEMISTRY JAPAN Vol. 76 ( 1 ) page： 37-44 2018.1

Synthesis of Heteroatom-Containing Curved pi-Conjugated Molecules Reviewed International journal

Hiroto, Satoru, Shinokubo, Hiroshi

Journal of Synthetic Organic Chemistry Japan Vol. 76 ( 1 ) page： 37 - 44 2018

Authorship：Last author,　Corresponding author Language：Japanese Publishing type：Research paper (scientific journal) Publisher：The Society of Synthetic Organic Chemistry, Japan

<p>Recently, π-conjugated molecules with curved-π surface have attracted considerable interest for their unique properties originating from their curved structures. However, most of them consist of only carbon and hydrogen atoms. In these situations, we have developed novel synthetic protocols for construction of distorted structures directly from 2D π-conjugated molecules under mild reaction conditions. By applying phenol and aniline oxidation methods, we have succeeded in the synthesis of highly distorted cyclophanes, π-extended heterohelicenes, and highly twisted porphyrin oligomers. Furthermore, we have succeeded in the synthesis of a nitrogen-embedded buckybowl as a novel bowl-shaped π-conjugated molecule with a pyrrolic nitrogen in its skeleton. These heteroatom containing curved-π conjugated molecules exhibit unique characteristics due to the combination of the curved structure with heteroatoms such as circularly polarized luminescence, strong C<sub>60</sub> binding, and near IR electrochromism. We believe that the chemistry of heteroatom containing curved-π conjugated molecules would enhance the potential of three-dimensional π-conjugated molecules for molecular materials.</p>

DOI： 10.5059/YUKIGOSEIKYOKAISHI.76.37

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Structures of the Heme Acquisition Protein HasA with Iron(III)-5,15-Diphenylporphyrin and Derivatives Thereof as an Artificial Prosthetic Group. Reviewed

Uehara H, Shisaka Y, Nishimura T, Sugimoto H, Shiro Y, Miyake Y, Shinokubo H, Watanabe Y, Shoji O

Angewandte Chemie (International ed. in English) Vol. 56 ( 48 ) page： 15279 - 15283 2017.11

Acid-Mediated Migration of Bromide in an Antiaromatic Porphyrinoid: Preparation of Two Regioisomeric Ni(II) Bromonorcorroles Reviewed

Kawashima Hiroyuki, Hiroto Satoru, Shinokubo Hiroshi

JOURNAL OF ORGANIC CHEMISTRY Vol. 82 ( 19 ) page： 10425 - 10432 2017.10

Shaping Antiaromatic -Systems by Metalation: Synthesis of a Bowl-Shaped Antiaromatic Palladium Norcorrole Reviewed

Yonezawa Tsubasa, Shafie Siham A., Hiroto Satoru, Shinokubo Hiroshi

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION Vol. 56 ( 39 ) page： 11822 - 11825 2017.9

Synthesis and Properties of meso-Arylated Corrphycenes. Reviewed

Nozawa R, Shinokubo H

Organic letters Vol. 19 ( 18 ) page： 4928 - 4931 2017.9

Design and Synthesis of Tunable Ligands with 4,4'-Bipyridyl as an Electron-Accepting Unit and Their Rhenium Complexes Reviewed

Kamatsuka Takuto, Shinokubo Hiroshi, Miyake Yoshihiro

ORGANOMETALLICS Vol. 36 ( 17 ) page： 3429 - 3434 2017.9

A synthesis of novel expanded porphyrinoids: Ni-II-induced nitrile cyclization of dicyanovinylene-bis (meso-aryl)dipyrrin Reviewed

Faialaga Nathan H., Ito Satoru, Shinokubo Hiroshi, Kim Younghoon, Kim Kimoon, Shin Ji-Young

DALTON TRANSACTIONS Vol. 46 ( 33 ) page： 10802 - 10808 2017.9

pi-Extended Dihydrophenazines with Three-State NIR Electrochromism Involving Large Conformational Changes Reviewed

Nagasaki Juri, Hiroto Satoru, Shinokubo Hiroshi

CHEMISTRY-AN ASIAN JOURNAL Vol. 12 ( 17 ) page： 2311 - 2317 2017.9

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Papers - SHINOKUBO, Hiroshi