Award type：Award from Japanese society, conference, symposium, etc.  Country：Japan

Award type：Award from Japanese society, conference, symposium, etc.  Country：Japan

Award type：Award from Japanese society, conference, symposium, etc.  Country：Japan

Country：Japan

受賞対象講演題目「熱可逆性超分子イオンゲルの調製と温度応答性制御」

Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1016/j.polymer.2021.123419

DOI： 10.1016/j.polymer.2021.123419

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Other Link： https://doi.org/10.1016/j.polymer.2021.123419

Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1021/acsapm.9b00861

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Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1039/c9ta01890e

DOI： 10.1039/c9ta01890e

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Other Link： https://pubs.rsc.org/en/content/articlepdf/2019/ta/c9ta01890e

Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1016/j.polymer.2017.03.010

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Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1021/acs.macromol.6b01867

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Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1002/marc.201500663

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PubMed

Authorship：Lead author,　Corresponding author   Language：Japanese   Publishing type：Research paper (scientific journal)  

DOI： https://doi.org/10.2324/gomu.90.9

Authorship：Lead author,　Corresponding author   Language：Japanese  

Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1021/ma502239w

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Authorship：Lead author,　Corresponding author   Language：Japanese   Publishing type：Research paper (scientific journal)  

DOI： 10.1678/rheology.43.125

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Authorship：Lead author,　Corresponding author  

Web of Science

Language：Japanese   Publishing type：Research paper (bulletin of university, research institution)  

Language：Japanese   Publishing type：Research paper (bulletin of university, research institution)  

Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1021/ma500517e

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Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1002/polb.23479

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Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1002/polb.23421

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Authorship：Corresponding author   Language：Japanese   Publishing type：Research paper (scientific journal)  

DOI： 10.1678/rheology.42.135

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Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1021/ma401820x

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Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

We report facile preparation of nanoporous thin films by rinsing out a metal salt from nanophase-separated hybrid films composed of a block copolymer and a water-soluble metal salt. Nanophase-separated hybrids were prepared by mixing polystyrene-b-poly(4-vinylpyridine) (PS-P4VP) and iron(III) chloride in a solvent of pyridine, followed by solvent-casting and thermal-annealing. Film samples with a thickness of ca. 100 nm were fabricated from the nanophase-separated hybrids by using a microtoming technique. Metal salts in the films were removed by immersion into water to fabricate nanopores. Morphological observations were conducted by using transmission electron microscopy (TEM). Ordered cylindrical nanopores were clearly observed in the thin films prepared from the water-immersed hybrids which originally present cylindrical nanodomains. These nanoporous films were modified by loading another metal salt, samarium(III) nitrate, into the nanopores on the basis of the coordination ability of P4VP tethered to the pore walls. The samples after loading treatment were evaluated by TEM observation and elemental analysis with energy dispersive X-ray spectroscopy.

DOI： 10.1021/la3042023

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PubMed

Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1021/ma301665e

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Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

Various supramacromolecular self-assembly mechanisms of complex polymer systems via non-covalent bonding interactions were summarized in this article. Basically, three types of systems were introduced. The first class is the morphological transition of block copolymer/homopolymer blends with hydrogen bonds (HBs) or block copolymer/metal salt hybrids via complex formation. Systematic morphological transition was observed upon the addition of a homopolymer or metal salt, depending on its composition of volume fraction. The second class consists of the formation of block copolymer-type supramacromolecules via hydrogen bonding between two chemical moieties connected at one end of each polymer chain, resulting in new nanophase-separated structures. As an advanced branch of this second class, new morphologies were observed in block copolymer/block copolymer blends with HBs. The third class is supramacromolecular gelation, which was observed for ABA triblock copolymer/C homopolymer or telechelic polymer/homopolymer blends, both including complementary electron donors/acceptors.

DOI： 10.1038/pj.2011.81

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Authorship：Lead author,　Corresponding author   Language：English  

Supramolecular polymer gels are precisely designed physical gels brought together by reversible secondary interactions to form three dimensional networks of melt macromolecules. Generally, they differ from supramolecular gels because they are comprised of polymers instead of low molecular weight compounds. Recently, much effort has focused on designing supramolecular polymer gels and related materials with excellent properties; indeed, improvements have been made in their supramolecular interactions, complementarity in the non-covalent bonding units, the nature of the macromolecular building blocks, and strand elasticity of supramolecular polymer networks. Owing to the precise molecular design, they represent nanophase separation and characteristic viscoelasticity. Here, we review supramolecular polymer gels in terms of molecular design, morphology, and rheology. We also discuss future directions in practical application of supramolecular polymer gels.

DOI： 10.1039/c2sm25144b

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Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

DOI： 10.1021/ma201440v

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Authorship：Lead author,　Corresponding author   Language：English   Publishing type：Research paper (scientific journal)  

Preparation of supramolecular polymer gels based on simple molecular design was demonstrated by blending carboxyl-terminated telechelic polymers and poly(ethyleneimine), where balance of an attractive force due to hydrogen bonding and a repulsive force induced by phase separation between polymers has been found as a key factor of supramolecular gelation.

DOI： 10.1039/c0sm01334j

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Authorship：Lead author,　Corresponding author   Language：Japanese  

Authorship：Lead author,　Corresponding author   Language：English   Publisher：Macromolecules  

We report a systematic study on preparation and morphology control of macroscopically homogeneous hybrid films composed of a block copolymer and a metal salt, where one block interacts with a metal salt by metal-to-ligand coordination. Hybrids were prepared by blending a polystyrene-b-poly(4- vinylpyridine) (PS - P4VP, Mn=37K, φs=0.79) block copolymer and iron(III) chloride (FeCl3) with changing the mole fraction of FeCl3. To prevent the rapid cross-linking formation between P4VP and FeCl3, pyridine as a polar solvent with the coordination ability was used at the solvent-casting stage, which turned out to be effective to prepare macroscopically homogeneous films with a large amount of FeCl3. Transmission electron microscopy and small-angle X-ray scattering measurements were carried out to observe the morphology of thermally annealed samples at the nanoscopic scale. It was revealed that simple two-phase nanostructures were observed due to homogeneously mixing of FeCl3 into a P4VP phase up to 0.9 mol equiv of FeCl3 to pyridine units in P4VP. This indicates FeCl3 works as a filler in a P4VP phase just as small homopolymers: domain expansion and morphology transition were observed as the amount of added FeCl3 increases. However, overflow of FeCl 3 was observed in the hybrid with an amount of 1.0 mol equiv of FeCl3. This is probably due to the saturation of incorporated FeCl3, indicating that morphology of the present system can be controlled by stoichiometric balance between 4-vinylpyridine units and FeCl 3. © 2010 American Chemical Society.

DOI： 10.1021/ma1007286

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Authorship：Lead author,　Corresponding author   Language：English   Publisher：Macromolecules  

Thermoreversible morphology transition from block-type supramacromolecules via hydrogen bonding was analyzed in an ionic liquid. Two macromolecular building blocks were designed to form a block-type supramacromolecule: one is a poly(3,4,5-trimethoxystyrene) with a small linker of poly(4-hydroxystyrene) on the end as a hydrogen-bonding proton donor, and the other is a poly(n-butyl acrylate) with a small linker of poly-(2-vinylpyridine) on the end as a hydrogen-bonding proton acceptor, both of which are soluble or at least dispersible in the ionic liquid. Measurements were taken every 20°C from lower to higher temperatures and vice versa. SAXS was used to reveal the thermo-reversible morphological transition from block-type supramacromolecules in an ionic liquid induced by hydrogen-bonding association-dissociation. The results show that this type of thermoreversible morphology transition in nanometer length scale could be achieved in similar systems if proper molecular design is performed.

DOI： 10.1021/ma901143k

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Language：Japanese  

Authorship：Lead author   Language：English   Publishing type：Research paper (scientific journal)  

Authorship：Lead author,　Corresponding author   Language：English   Publisher：Macromolecules  

A series of supramacromolecular ion gels were prepared from blends of a poly(2-vinylpyridine)-b-poly(ethyl acrylate)-b-poly(2-vinylpyridine) (VEAV) triblock copolymer and a poly(4-hydroxystyrene) (H) homopolymer in an ionic liquid. The VEAV concentration was held at 10 wt %, and the H concentration was varied from 0 to 8 wt %. The solvent was the room temperature ionic liquid 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl) imide (EMITFSI). Above 160°C all samples formed homogeneous solutions, but upon cooling gels were formed due to increased hydrogen bonds between the V blocks and H cross-linkers. The gelation mechanism was investigated in detail by rheology and small-angle X-ray scattering. The gel point (gel-liquid transition temperature) increased with the concentration of the cross-linkers. The dynamic moduli, G′ and G″, showed excellent time-temperature superposition, and gave master curves extending over 15 orders of magnitude in reduced frequency. The shift factors aT showed the same strong temperature dependence for all the samples, which is attributed to the increasing number of hydrogen bonds between a given V block and H cross-linker upon cooling below the gel point. The gel quality was assessed in terms of the modulus value, Gx, the sharpness of the change in dynamic moduli with temperature near the gel point, and the minimum value of tan δ in the gel regime. By all three measures the best gel was formed at the mole ratio closest to 1:1 of pyridine:phenol units, i.e., stoichiometric balance. Furthermore, the maximum value of Gx corresponded to 50% of the EA blocks being elastically effective, consistent with expectation given the tendency for midblocks to loop back into the same micelle. A gel-like response was also obtained upon mixing 10% of a poly(2-vinylpyridine)-b-poly(ethyl acrylate) (VEA) diblock copolymer and H homopolymers in EMITFSI. However, in this case the rheological properties resulted from congestion of micelles rather than bridging chains. Small angle X-ray scattering revealed the presence of a nanophase-separated state, but without any significant change on traversing the gel point, or between diblock and triblock samples. © 2009 American Chemical Society.

DOI： 10.1021/ma900820g

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Authorship：Lead author,　Corresponding author   Language：English   Publisher：Polymer  

This review paper summarizes recent advances in self-assembly of complex polymers, focusing on three characteristic polymeric systems. The first is star-branched polymers of the ABC type, the second one consists of multiblock terpolymers with different chain lengths, while the third comprises supramacromolecular assembly systems with hydrogen and ionic bonding interactions between different polymer species. A quasicrystalline tiling structure with mesoscopic length scale has been found for the first star polymer system as well as the periodic Archimedean tiling structures, and moreover three-dimensional Zincblende network structure has been discovered. Furthermore the hierarchical structures having two length scales have been also found for the ABC star molecules whose chain length ratios, that is, A/B and/or A/C are larger than approximately five. Hierarchical structures with double periodicity have been observed for the hexablock and undecablock terpolymers and it has been revealed that their morphology changes systematically depending on composition of polymeric species. Poly(4-hydroxystyrene) (H) homopolymer was found to be dissolved into microdomain of poly(2-vinylpyridine) formed by poly(styrene-b-2-vinylpyridine) due to hydrogen bonding interaction, resulting in the origin of morphological transitions depending on the composition of H homopolymer added. Hierarchical structures possessing double periodicity have been found for poly(isoprene-b-2-vinylpyridine)/poly(styrene-b-4-hydroxystyrene) blends depending on both volume fractions of component polymers and blend ratio. Blends of different homopolymers with several complementary nucleotides or acid/base moieties on chain ends have been confirmed to show nanophase-separated structures as a result of successful formation of "supramacromolecules". © 2009 Elsevier Ltd. All rights reserved.

DOI： 10.1016/j.polymer.2009.02.047

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Authorship：Lead author,　Corresponding author   Language：English   Publisher：Macromolecules  

We report a systematic study on nanophase-separated structures from block- and graft-type supramacromolecules via acid-base complexation, where supramacromolecules are termed as supramolecules composed of a pair of macromolecules with complementary noncovalent bonding moieties. Block- or graft-type supramacromolecules were built up by blending component polymers, that is, sulfonic acid-terminated polystyrene (PS-SO3H, Mn = 19 k) or polystyrene-block-poly(4-styrenesulfonic acid) (PS-P(SSO 3H), Mn =23k) with primary amine-terminated polyisoprene (PI-NH 2, Mn = 17 k). Self-assembled nanostructures of the blends were confirmed complementarity by transmission electron microscopy and small-angle X-ray scattering. At larger acid/base molar ratio, the blends show comparatively ordered nanophase-separated structures without macrophase-separated large PS domain. Morphological transition controlled by composition has occurred in the blends of PS-P(SSO3H)/PINH2 as ordinary block copolymers show, though the blends of PS-SO3H/PI-NH2 showed macrophase separation at excess ratio of PI-NH2 to PS-SO 3H. The difference in composition dependence of morphology between two blend series is resulted from stoichiometric effects of sulfonic acid vs amine. Therefore, PS-P(SSO3H) is more useful to build up various supramacromolecular complexes with PI-NH2 than PS-SO3H just by changing the molar ratios of component polymers, that is, multiple noncovalent bonding can be found more advantageous, resulting in conforming graft-type supramacromolecules, not a block-type supramacromolecule from. PI-NH2 and PS-SO3H. © 2008 American Chemical Society.

DOI： 10.1021/ma801661c

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Authorship：Lead author,　Corresponding author   Language：English   Publisher：Macromolecules  

We report the thermoreversible viscoelastic properties of a supramolecular ion gel. Two building blocks were used to form "supramacromolecules". An ABA triblock copolymer (Mn = 50 000, poly(2-vinylpyridine)-b- poly(ethyl acrylate)-b-poly(2-vinylpyridine)) (P2VP-PEA-P2VP), with a mole ratio of 0.1/0.8/0.1 as a telechelic polymer, and a poly(4-hydroxystyrene) (PHS) homopolymer, with Mn = 6600 as a connector, form a physical gel via hydrogen bonding between P2VP and PHS. The thermally stable, hydrophobic ionic liquid 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide (EMITFSI) provided a good solvent medium for PEA from room temperature up to at least 160°C. A solution containing 10 wt % P2VP-PEA-P2VP and 4% PHS was a liquid at elevated temperatures but on cooling formed a network at 141.5°C. Dynamic shear moduli obtained as a function of frequency at various temperatures from 30 to 160°C could be superposed to form excellent master curves, with a distinct plateau modulus extending over more than 11 orders of magnitude in frequency. The longest relaxation time inferred from the time-temperature superposition shift factors showed a similar 11 order of magnitude increase on cooling. This remarkable temperature sensitivity of the supramacromolecular ion gel is attributed to the formation of multiple hydrogen bonds between a given P2VP block and PHS cross-linker. A hydrogen bond energy of 13 kJ/mol was estimated from temperature-dependent FTIR measurements, and a straightforward analysis yielded an estimate of the number of hydrogen bonds per P2VP block as a function of temperature. This system is distinct from other supramolecular hydrogen-bonded polymers, and from hydrophobically modified associating polymers, in that below the gelation temperature the number of physical cross-links is independent of temperature, but the strength of each association, namely, the number of active hydrogen bonds within a particular cross-link site, increases strongly on cooling. © 2008 American Chemical Society.

DOI： 10.1021/ma800739c

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Authorship：Lead author,　Corresponding author   Language：English   Publisher：Macromolecules  

Morphological transition of two types of multiblock terpolymers with composition has been investigated. One is undecablock terpolymers of the PISISISISIP type, while the other is hexablock terpolymers of the PISISI type, where P, I, and S denote poly(2-vinylpyridine), polyisoprene, and polystyrene, respectively. These polymer samples were prepared on the basis of anionjc polymerization method. The volume fractions of P, φp, of the former are 0.08, 0.21, 0.53, whereas those of the latter are 0.64, 0.75, and 0.87. Nanophase-separated structures were observed by TEM and SAXS, and it was confirmed that their hierarchical morphology transforms from spheres-in-lamellae structure into cylinders-in-lamellae, lamellae-in-lamella, and coaxial cylinderical structures and finally into onionlike spherical structure with increasing volume fraction of the P component. From these results, it has been found that morphological transition of multiblock terpolymers takes place obeying conventional rule, i.e., the domain shape of P component varies as sphere-cylinder-lamella-matrix as φp increases with keeping hierarchical lamellar structure from I and S. © 2007 American Chemical Society.

DOI： 10.1021/ma070155s

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Language：Japanese   Publishing type：Research paper (scientific journal)  

Authorship：Lead author,　Corresponding author   Language：English   Publisher：Polymer Journal  

Neutron reflectometry is a very powerful and essential technique for the studies on material interfaces due lo its high spatial resolution, ∼a few tenths of nm, along the depth direction. The use of neutron as a probe is a big advantage for structural analysis on soft-materials, since the scattering contrast can be highly enhanced in hydrogenous materials such as polymers, surfactants, lipids, proteins, etc.. without big changes in their physical and chemical properties by substituting all or part of the hydrogen atoms in the molecules with deuterium (a deuterium labeling method). Furthermore, the neutron reflectometry can explore deeply-buried interfaces such as solid/liquid interfaces in a non-destruetive way, and make in situ measurements combined with various sample environments due to its high transmission to the materials. In this article, the neutron reflectometry is reviewed from the standpoint of researches on interfacial structures of the thin films of polymer and lipid, and its future prospects at a high-intensity pulsed-neutron source are presented. © 2007 The Society of Polymer Science.

DOI： 10.1295/polymj.PJ2007113

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Authorship：Lead author,　Corresponding author   Language：English   Publisher：Physica B: Condensed Matter  

Segmental distribution of polystyrene blocks in lamellar microphase-separated poly(styrene-block-2-vinylpyridine) (SP) with wide composition distribution was investigated by neutron reflectivity measurements using deuterium-labeled polymers. Block copolymers with wide composition distribution were produced by mixing three monodispersed parent block copolymers, which were synthesized by an anionic polymerization method to have the same total molecular weight but with different volume fractions. The block copolymer blends whose overall S/P ratio is 0.5/0.5 were found to form a uniform lamellar structure, where lamellae were highly oriented along the direction parallel to the film surface and the interfacial thickness was evaluated as 40 Å. It was clarified that a shorter block chain in the microdomain is localized at the domain boundary, while a longer one has a peak at the center of microdomain in its segmental distribution profile. © 2006 Elsevier B.V. All rights reserved.

DOI： 10.1016/j.physb.2006.05.303

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Authorship：Lead author,　Corresponding author   Language：English   Publisher：Macromolecules  

The effect of composition distribution on microphase-separated structures of AB diblock and BAB triblock copolymers was investigated at the molecular level by measurements of neutron reflectivity. Monodispersed three poly(styrene)-d 8-block-poly(2-vinylpyridine) (DP) and three labeled triblock copolymers (PDP) and unlabeled counterparts were synthesized by a living anionic polymerization process designed to yield constant molecular weight with different volume fractions. The selective labeling method employs the blending of copolymers for a segmental distribution study while the labeled polymers are mixed for an interfacial study. Scattering length density profiles were observed by neutron reflectivity measurements for blended thin films produced by spin-coating and successive thermal annealing. It was confirmed that the blended thin films exhibit simple alternating lamellar structures, an observation consistent with the observed structures of bulk specimens. The localization phenomenon of longer and shorter block chains was also investigated. Longer block chains are generally localized at the center of the domains while the shorter block chains are localized near the domain interface as suggested by previous morphological observations. Interfacial thickness increases with an increase in composition distribution index for both diblock and triblock systems. The incremental increase for the triblock system is larger than that of the diblock system. © 2006 American Chemical Society.

DOI： 10.1021/ma061487k

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Authorship：Lead author,　Corresponding author   Language：English   Publisher：Physical Review Letters  

A new nanophase-separated structure with parallel double periodicity has been identified for an undecablock terpolymer in bulk. The polymer includes two long poly(2-vinypyridine) (P) chains on each end, with five short polyisoprene (I) and four short polystyrene (S) chains at the center. This polymer exhibits a hierarchical lamellar structure with two crystallographic periods: 88 nm and 16 nm. The 88 nm period includes one thick P lamella and five thin I-S-I-S-I lamellae, of extremely high orientation. © 2006 The American Physical Society.

DOI： 10.1103/PhysRevLett.97.098301

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PubMed

Authorship：Lead author,　Corresponding author   Language：English   Publisher：Biomacromolecules  

Control of nanostructure formation by a diblock-type supramacromolecule via biocomplementary hydrogen bonding has been achieved. Two different homopolymers, poly(4-trimethylsilylstyrene) and poly(styrene-d8), that are end-decorated with complementary oligonucleotides, i.e., thymidine phosphates and deoxyadenosine phosphates, were prepared by using the phosphoramidite method and blended successively. Association behavior in a blend solution was examined with NMR, and a cast bulk film obtained from the solution has been confirmed to show a nanophase-separated structure by transmission electron microscopy and X-ray scattering. Suppression of this nanostructure formation of a block-type supramacromolecule was also attained by adding a smaller agent as an inhibitor. © 2006 American Chemical Society.

DOI： 10.1021/bm0602280

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Authorship：Last author   Language：Japanese   Publisher：Kobunshi Ronbunshu  

Studies on self-assembled multiphase structures of block- and graft polymers in condensed systems were reviewed. The article includes six chapters. Individual chapters are as follows: Chap. 1, Introduction; Chap. 2; history of nanophase-separated structure; Chap. 3, preparation and characterization of polymer samples; Chap. 4, morphological observations; Chap. 5; several properties; and Chap. 6, summary. The main chapter is Chap. 4. It consists of 1) morphological transition with composition, 2) domain spacing and chain dimensions of component polymers in bulk, 3) phase transition depending on external fields and microdomain interface, and 4) new hierarchical structures from newly-designed polymers. Basically amorphous polymers were treated either in glassy state or in rubbery state to avoid confusion. Amphiphilic molecules or polyelectrolytes in solutions and micelle formation of block copolymers in selective solvents were excluded due to lack of space though such fields have potential importance. Two schemes and 16 figures were used to explain research achievements and about 100 references were cited.

DOI： 10.1295/koron.63.205

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Language：English   Publishing type：Research paper (scientific journal)  

Language：English   Publishing type：Research paper (scientific journal)  

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Authorship：Lead author   Language：English   Publishing type：Research paper (scientific journal)  

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Authorship：Lead author   Language：English   Publishing type：Research paper (scientific journal)  

Language：English   Publishing type：Research paper (scientific journal)  

Total pages：14   Language：Japanese Book type：Scholarly book

Language：Japanese

PartⅡ 14章「フォトニック材料」を担当

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セクション「相分離型超分子ソフト材料」を担当
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Event date： 2023.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：香川大学 幸町キャンパス   Country：Japan  

Event date： 2023.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：香川大学 幸町キャンパス   Country：Japan  

Event date： 2023.7

Language：English   Presentation type：Oral presentation (general)  

Venue：Makuhari Messe   Country：Japan  

Event date： 2023.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：Ｇメッセ群馬   Country：Japan  

Event date： 2022.12

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：三重大学三翠ホール   Country：Japan  

Event date： 2022.12

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：三重大学三翠ホール   Country：Japan  

Event date： 2022.12

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：三重大学三翠ホール   Country：Japan  

Event date： 2022.11

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：アクティブリゾーツ宮城蔵王   Country：Japan  

Event date： 2022.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：北海道大学 札幌キャンパス   Country：Japan  

Event date： 2022.3

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：オンライン   Country：Japan  

Event date： 2021.11

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：九州大学稲盛財団記念館稲盛ホール（オンライン併用）   Country：Japan  

Event date： 2021.11

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：九州大学稲盛財団記念館稲盛ホール（オンライン併用）   Country：Japan  

Event date： 2021.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：オンライン   Country：Japan  

Event date： 2020.11

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：オンライン   Country：Japan  

Event date： 2020.5

Language：Japanese   Presentation type：Poster presentation  

Venue：福岡国際会議場（博多）   Country：Japan  

Event date： 2020.5

Language：Japanese   Presentation type：Poster presentation  

Venue：福岡国際会議場（博多）   Country：Japan  

Event date： 2020.5

Language：Japanese   Presentation type：Poster presentation  

Venue：名古屋プライムセントラルタワー（名古屋）   Country：Japan  

Event date： 2020.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：名古屋プライムセントラルタワー（名古屋）   Country：Japan  

Event date： 2020.5

Language：Japanese   Presentation type：Poster presentation  

Venue：東京大学生産技術研究所（東京）   Country：Japan  

Event date： 2016.3

Language：English   Presentation type：Oral presentation (general)  

Country：United States  

Event date： 2016.3

Language：English   Presentation type：Poster presentation  

Country：United States  

Event date： 2016.3

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2015.3

Language：English   Presentation type：Oral presentation (general)  

Country：United States  

Event date： 2014.12

Language：English   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2014.11

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2014.10

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：福井   Country：Japan  

Event date： 2014.10

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：福井（福井市地域交流プラザ）   Country：Japan  

Event date： 2014.10

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2014.10

Language：Japanese   Presentation type：Poster presentation  

Venue：東京（タワーホール船堀）   Country：Japan  

Event date： 2014.10

Language：English   Presentation type：Poster presentation  

Country：United States  

Event date： 2014.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：長崎（長崎大学）   Country：Japan  

Event date： 2014.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：長崎（長崎大学）   Country：Japan  

Event date： 2014.5

Language：Japanese   Presentation type：Poster presentation  

Venue：名古屋（名古屋国際会議場）   Country：Japan  

Event date： 2014.5

Language：Japanese   Presentation type：Poster presentation  

Venue：名古屋（名古屋国際会議場）   Country：Japan  

Event date： 2014.5

Language：Japanese   Presentation type：Poster presentation  

Venue：名古屋（名古屋国際会議場）   Country：Japan  

Event date： 2014.5

Language：Japanese   Presentation type：Poster presentation  

Venue：名古屋（名古屋国際会議場）   Country：Japan  

Event date： 2014.5

Language：Japanese   Presentation type：Poster presentation  

Venue：名古屋（名古屋国際会議場）   Country：Japan  

Event date： 2014.5

Language：Japanese   Presentation type：Poster presentation  

Venue：東京（東京大学）   Country：Japan  

Event date： 2014.5

Language：Japanese   Presentation type：Poster presentation  

Venue：東京（東京大学）   Country：Japan  

Event date： 2014.3

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：名古屋（名古屋大学）   Country：Japan  

Event date： 2014.3

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：名古屋（名古屋大学）   Country：Japan  

Event date： 2014.3

Language：Japanese   Presentation type：Poster presentation  

Venue：つくば（つくば国際会議場）   Country：Japan  

Event date： 2014.3

Language：Japanese   Presentation type：Poster presentation  

Venue：つくば（つくば国際会議場）   Country：Japan  

Event date： 2014.3

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2014.3

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2014.3

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2014.1

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：東京（東京大学）   Country：Japan  

Event date： 2014.1

Language：Japanese   Presentation type：Poster presentation  

Venue：東京（東京大学）   Country：Japan  

Event date： 2013.11

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：浜松（静岡大学工学部）   Country：Japan  

Event date： 2013.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：米沢（山形大学工学部）   Country：Japan  

Event date： 2013.9

Language：Japanese   Presentation type：Poster presentation  

Venue：米沢（山形大学工学部）   Country：Japan  

Event date： 2013.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：金沢（金沢大学）   Country：Japan  

Event date： 2013.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：金沢（金沢大学）   Country：Japan  

Event date： 2013.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：金沢（金沢大学）   Country：Japan  

Event date： 2013.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：金沢（金沢大学）   Country：Japan  

Event date： 2013.7

Language：Japanese   Presentation type：Poster presentation  

Venue：広島（広島国際会議場）   Country：Japan  

Event date： 2013.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：京都（京都国際会館）   Country：Japan  

Event date： 2013.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：京都（京都国際会館）   Country：Japan  

Event date： 2013.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：京都（京都国際会館）   Country：Japan  

Event date： 2013.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：京都（京都国際会館）   Country：Japan  

Event date： 2013.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：京都（京都国際会館）   Country：Japan  

Event date： 2013.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：京都（京都テルサ）   Country：Japan  

Event date： 2013.3

Language：Japanese   Presentation type：Poster presentation  

Venue：つくば（エポカルつくば）   Country：Japan  

Event date： 2013.3

Language：Japanese   Presentation type：Poster presentation  

Venue：つくば（エポカルつくば）   Country：Japan  

Event date： 2013.3

Language：English   Presentation type：Poster presentation  

Country：China  

Event date： 2013.1

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：東京（東京大学）   Country：Japan  

Event date： 2013.1

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：東京（東京大学）   Country：Japan  

Event date： 2012.12

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2012.12

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2012.11

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：名古屋（名古屋工業大学）   Country：Japan  

Event date： 2012.11

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：名古屋（名古屋工業大学）   Country：Japan  

Event date： 2012.9

Language：English   Presentation type：Oral presentation (general)  

Venue：名古屋   Country：Japan  

Event date： 2012.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：名古屋   Country：Japan  

Event date： 2012.9

Language：Japanese   Presentation type：Poster presentation  

Venue：名古屋   Country：Japan  

Event date： 2012.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：名古屋   Country：Japan  

Event date： 2012.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：名古屋   Country：Japan  

Event date： 2012.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：名古屋   Country：Japan  

Event date： 2012.8 - 2012.9

Language：Japanese   Presentation type：Poster presentation  

Venue：三重県津   Country：Japan  

Event date： 2012.8 - 2012.9

Language：Japanese   Presentation type：Poster presentation  

Venue：三重県津   Country：Japan  

Event date： 2012.8 - 2012.9

Language：Japanese   Presentation type：Poster presentation  

Venue：三重県津   Country：Japan  

Event date： 2012.8 - 2012.9

Language：Japanese   Presentation type：Poster presentation  

Venue：三重県津   Country：Japan  

Event date： 2012.6

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：江別（酪農学園大学）   Country：Japan  

Event date： 2012.5

Language：English   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2012.5

Language：Japanese   Presentation type：Poster presentation  

Venue：横浜(パシフィコ横浜)   Country：Japan  

Event date： 2012.5

Language：Japanese   Presentation type：Poster presentation  

Venue：横浜(パシフィコ横浜)   Country：Japan  

Event date： 2012.5

Language：Japanese   Presentation type：Poster presentation  

Venue：横浜(パシフィコ横浜)   Country：Japan  

Event date： 2012.5

Language：English   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2012.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：東京（東京大学）   Country：Japan  

Event date： 2012.5

Language：Japanese   Presentation type：Poster presentation  

Venue：東京（東京大学）   Country：Japan  

Event date： 2012.3

Language：Japanese   Presentation type：Poster presentation  

Venue：つくば（エポカルつくば）   Country：Japan  

Event date： 2012.3

Language：Japanese   Presentation type：Poster presentation  

Venue：つくば（エポカルつくば）   Country：Japan  

Event date： 2012.3

Language：Japanese   Presentation type：Poster presentation  

Venue：つくば（エポカルつくば）   Country：Japan  

Event date： 2012.3

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：名古屋（豊田工業大学）   Country：Japan  

Event date： 2012.3

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：名古屋（豊田工業大学）   Country：Japan  

Event date： 2011.11

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2011.11

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2011.11

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2011.11

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：長野   Country：Japan  

Event date： 2011.11

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：長野   Country：Japan  

Event date： 2011.10

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：群馬県桐生   Country：Japan  

Event date： 2011.10

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：群馬県桐生   Country：Japan  

Event date： 2011.9

Language：Japanese   Presentation type：Poster presentation  

Venue：岡山   Country：Japan  

Event date： 2011.9

Language：Japanese   Presentation type：Poster presentation  

Venue：岡山   Country：Japan  

Event date： 2011.9

Language：Japanese   Presentation type：Poster presentation  

Venue：岡山   Country：Japan  

Event date： 2011.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：岡山   Country：Japan  

Event date： 2011.9

Language：Japanese   Presentation type：Poster presentation  

Venue：三重県三重郡   Country：Japan  

Event date： 2011.9

Language：Japanese   Presentation type：Poster presentation  

Venue：三重県三重郡   Country：Japan  

Event date： 2011.9

Language：Japanese   Presentation type：Poster presentation  

Venue：三重県三重郡   Country：Japan  

Event date： 2011.7

Language：Japanese   Presentation type：Poster presentation  

Venue：つくば   Country：Japan  

Event date： 2011.7

Language：Japanese   Presentation type：Poster presentation  

Venue：つくば   Country：Japan  

Event date： 2011.7

Language：Japanese   Presentation type：Poster presentation  

Venue：つくば   Country：Japan  

Event date： 2011.5

Language：Japanese   Presentation type：Poster presentation  

Venue：大阪   Country：Japan  

Event date： 2011.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：大阪   Country：Japan  

Event date： 2011.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：大阪   Country：Japan  

Event date： 2011.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：大阪   Country：Japan  

Event date： 2011.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：大阪   Country：Japan  

Event date： 2011.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：大阪   Country：Japan  

Event date： 2011.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：京都   Country：Japan  

Event date： 2011.5

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2010.12

Language：English   Presentation type：Poster presentation  

Country：United States  

Event date： 2010.12

Language：English   Presentation type：Poster presentation  

Country：United States  

Event date： 2010.12

Language：English   Presentation type：Oral presentation (general)  

Country：United States  

Event date： 2010.11

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2010.11

Language：Japanese   Presentation type：Poster presentation  

Venue：名古屋   Country：Japan  

Event date： 2010.11

Language：Japanese   Presentation type：Poster presentation  

Venue：名古屋   Country：Japan  

Event date： 2010.11

Language：Japanese   Presentation type：Poster presentation  

Venue：名古屋   Country：Japan  

Event date： 2010.11

Language：Japanese   Presentation type：Poster presentation  

Venue：大阪   Country：Japan  

Event date： 2010.11

Language：Japanese   Presentation type：Poster presentation  

Venue：大阪   Country：Japan  

Event date： 2010.11

Language：English   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2010.11

Language：English   Presentation type：Oral presentation (general)  

Venue：豊橋   Country：Japan  

Event date： 2010.10

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：仙台   Country：Japan  

Event date： 2010.10

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：仙台   Country：Japan  

Event date： 2010.9

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2010.9

Language：Japanese   Presentation type：Poster presentation  

Country：Japan  

Event date： 2010.9

Language：Japanese   Presentation type：Poster presentation  

Venue：愛知県蒲郡   Country：Japan  

Event date： 2010.9

Language：Japanese   Presentation type：Poster presentation  

Venue：愛知県蒲郡   Country：Japan  

Event date： 2010.8

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2010.5

Language：Japanese   Presentation type：Poster presentation  

Country：Japan  

Event date： 2010.5

Language：Japanese   Presentation type：Poster presentation  

Country：Japan  

Event date： 2010.5

Language：Japanese   Presentation type：Poster presentation  

Country：Japan  

Event date： 2010.5

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2010.5

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2010.3

Language：English   Presentation type：Poster presentation  

Country：United States  

Event date： 2010.3

Language：English   Presentation type：Oral presentation (general)  

Country：United States  

Event date： 2010.3

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2010.3

Language：Japanese   Presentation type：Poster presentation  

Venue：つくば   Country：Japan  

Event date： 2009.11

Language：Japanese   Presentation type：Poster presentation  

Venue：名古屋   Country：Japan  

Event date： 2009.11

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2009.11

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2009.10

Language：English   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2009.10

Language：English   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2009.10

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2009.9

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2009.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：熊本   Country：Japan  

Event date： 2009.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：熊本   Country：Japan  

Event date： 2009.9

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：熊本   Country：Japan  

Event date： 2009.9

Language：Japanese   Presentation type：Poster presentation  

Venue：岐阜   Country：Japan  

Event date： 2009.9

Language：Japanese   Presentation type：Poster presentation  

Venue：岐阜   Country：Japan  

Event date： 2009.5

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2009.5

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2009.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：神戸   Country：Japan  

Event date： 2009.5

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：神戸   Country：Japan  

Event date： 2009.1

Language：English   Presentation type：Oral presentation (invited, special)  

Country：Japan  

Event date： 2008.11

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2008.10

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2008.9

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2008.8

Language：Japanese   Presentation type：Poster presentation  

Country：Japan  

Event date： 2008.7

Language：English   Presentation type：Oral presentation (general)  

Event date： 2008.5

Language：Japanese   Presentation type：Poster presentation  

Country：Japan  

Event date： 2008.3

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2008

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2007.12

Language：English   Presentation type：Poster presentation  

Country：Japan  

Event date： 2007.11

Language：Japanese   Presentation type：Oral presentation (general)  

Venue：津   Country：Japan  

Event date： 2007.5

Language：English   Presentation type：Oral presentation (general)  

Event date： 2006.5

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2006.4

Language：English   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2005.9

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2005.5

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2005.1

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2004.9

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2004.9

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2004.5

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2003.9

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

Event date： 2003.5

Language：Japanese   Presentation type：Oral presentation (general)  

Country：Japan  

https://www.jstage.jst.go.jp/article/fiber/72/1/72_P-13/_article/-char/ja/

https://npc.e-manager.jp/actibook-file/index/000/000/178/HTML5/pc.html/?memberNum=0&groupNum=1G#/page/1

http://www.ceramic.or.jp/ihensyub/topics/topics2014.11.pdf

Applicant：東海国立大学機構

Application no：JP2021-056359   Date applied：2021.3

Announcement no：2022-153700  Date announced：2022.10

Country of applicant：Domestic   Country of acquisition：Domestic

Applicant：東海国立大学機構,日本ゼオン

Application no：PCT/JP2021/004159  Date applied：2021.2

Announcement no：WO 2021/171954  Date announced：2021.9

Country of applicant：Foreign country   Country of acquisition：Foreign country

Applicant：東海国立大学機構,日本ゼオン

Application no：PCT/JP2021/004159  Date applied：2021.2

Announcement no：WO 2021/171954  Date announced：2021.9

Country of applicant：Foreign country   Country of acquisition：Foreign country

Applicant：東海国立大学機構,トヨタ自動車

Application no：2020-212382  Date applied：2020.12

Announcement no：2022-098788  Date announced：2022.7

Country of applicant：Domestic   Country of acquisition：Domestic

Applicant：東海国立大学機構,トヨタ自動車

Application no：2020-196798  Date applied：2020.11

Announcement no：2022-085223  Date announced：2022.6

Country of applicant：Domestic   Country of acquisition：Domestic

Applicant：東海国立大学機構,トヨタ自動車

Application no：2020-167152  Date applied：2020.10

Announcement no：2022-059412  Date announced：2022.4

Country of applicant：Domestic   Country of acquisition：Domestic

Applicant：トヨタ自動車株式会社、国立大学法人名古屋大学

Application no：KR10-2019-0130351  Date applied：2019.10

Date announced：2021.11

Patent/Registration no：10-2330170  Date registered：2021.11 

Country of applicant：Foreign country  

Applicant：法人名大,トヨタ自動車

Application no：CN201910999451  Date applied：2019.10

Announcement no：CN111092250  Date announced：2020.5

Country of applicant：Foreign country   Country of acquisition：Foreign country

Applicant：法人名大,トヨタ自動車

Application no：US16/656,908  Date applied：2019.10

Announcement no：US 2020/0136164  Date announced：2020.4

Patent/Registration no：11322764  Date registered：2022.5 

Country of applicant：Foreign country   Country of acquisition：Foreign country

Applicant：法人名大,トヨタ自動車

Application no：EP19204160  Date applied：2019.10

Announcement no：3644420  Date announced：2020.4

Country of applicant：Foreign country   Country of acquisition：Foreign country

Applicant：東海国立大学機構

Application no：PCT/2019/ 029509  Date applied：2019.7

Announcement no：WO 2020/022503  Date announced：2020.1

Country of applicant：Foreign country   Country of acquisition：Foreign country