Faculty Profiles - HIBINO, Takashi

Papers - HIBINO, Takashi

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Electrochemical production of methanol and hydrogen from biomass waste Reviewed

Zichun Xiong, Kazuyo Kobayashi, Aki Miyawaki, Shinya Teranishi, Takashi Hibino

Electrochemistry Communications page： 107862 2025.1

Electro-oxidative extraction of methanol from lignin using a three-dimensional graphite anode Invited Reviewed

Zichun Xiong, Kazuyo Kobayashi, Aki Miyawaki, Shinya Teranishi, Yoshiharu Sawada, Takashi Hibino

ChemElectroChem page： e202400464 2024.11

総説：廃棄バイオマスの電解酸化によるエネルギー・資源変換

日比野高士

触媒 Vol. 66 ( 6 ) 2024.12

総説：廃棄バイオマスを利用した燃料電池と電気分解

日比野高士

日本化学会「化学と教育」 Vol. 72 ( 6 ) 2024.6

Electrochemical extraction of methanol from lignin under mild conditions Reviewed

Takashi Hibino, Kazuyo Kobayashi, Dongwen Zhou, Siyuan Chen, Anatoly Zinchenko, Shinya Teranishi, Aki Miyawaki, Yoshiharu Sawada

Applied Catalysis B: Environmental Vol. 341 page： 123328 2023.9

Alternating current electrolysis for individual synthesis of methanol and ethane from methane in a thermo-electrochemical cell Reviewed

Takashi Hibino, Kazuyo Kobayashi, Masahiro Nagao, Dongwen Zhou, Siyuan Chen, Yuta Yamamoto

ACS Catalysis Vol. 13 page： 8890 - 8901 2023.6

Two-stage electrolysis of H2O and CO2 to methanol: CO2-to-methane reduction at the cathode and subsequent methane-to-methanol oxidation at the anode Reviewed

Hibino Takashi, Kobayashi Kazuyo, Nagao Masahiro, Dongwen Zhou, Siyuan Chen

JOURNAL OF MATERIALS CHEMISTRY A Vol. 10 ( 42 ) page： 22718 - 22729 2022.11

Authorship：Lead author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：Journal of Materials Chemistry A

Co-electrolysis of H2O and N/C sources to valuable chemicals has the potential to contribute to global warming mitigation. We here report the electrochemical conversion of H2O and CO2 into methanol in a gas flow system at temperatures between 100 and 200 °C. CO2 was reduced to methane with voltage-boosted H2 at a Ru/C cathode. Introduced Fe2O3 nanoparticles promoted the adsorption and activation of CO2 on the surface of Ru because of their high redox activity. Methane was oxidized to methanol through the formation of ˙CH3 and active oxygen species at a Pt anode. The addition of Au to the anode enhanced the selectivity toward methanol by reducing the activity of Pt in the complete oxidation of methanol. Combining these processes with gas penetration into the electrolyte membrane enabled the synthesis of methanol from H2O and CO2, with a maximum faradaic efficiency of 54%. This work establishes a methodology for providing a good balance between the activity and selectivity of electrodes for the CO2 reduction reaction.

DOI： 10.1039/d2ta04011e

Web of Science

Scopus

Solid oxide fuel cell using plastic waste directly as fuel Reviewed

Takashi Hibino, Kazuyo Kobayashi, Takuma Hitomi

Chemistry Letters Vol. 50 ( 10 ) page： 1729 - 1732 2021.10

Biomass solid oxide fuel cell using solid weed waste as fuel Reviewed

Takashi Hibino, Kazuyo Kobayashi, Takuma Hitomi

Electrochimica Acta Vol. 388 page： 138681 2021.8

Solid oxide fuel cell using municipal solid waste directly as fuel: biomass, resin, plastic, and food waste Reviewed

Takashi Hibino, Kazuyo Kobayashi, Shinya Teranishi, Takuma Hitomi

ACS Sustainable Chemistry & Engineering Vol. 9 ( 8 ) page： 3124 - 3136 2021.3

A NiRhS fuel cell catalyst-lessons from hydrogenase Reviewed

Seiji Ogo, Tatsuya Ando, Le Tu Thi Minh, Yuki Mori, Takahiro Matsumoto, Takeshi Yatabe, Ki-Seok Yoon, Yukio Sato, Takashi Hibino, Kenji Kaneko

Chemical Communications Vol. 56 ( 79 ) page： 11787 - 11790 2020.10

Ionic conductive and photocatalytic properties of cementitious materials: calcium silicate hydrate and calcium aluminoferrite Reviewed

Masahiro Nagao, Kazuyo Kobayashi, Yongcheng Jin, Ippei Maruyama, Takashi Hibino

Journal of Materials Chemistry A Vol. 8 ( 30 ) page： 15157 - 15166 2020.8

Fuel cell and electrolyzer using plastic waste directly as fuel Reviewed

Tetsuya Hori, Kazuyo Kobayashi, Shinya Teranishi, Masahiro Nagao, Takashi Hibino

Waste Management Vol. 102 page： 30 - 39 2020.2

A cellulose electrolysis cell with metal-free carbon electrodes Reviewed

Yaorong Li, Masahiro Nagao, Kazuyo Kobayashi, Yongcheng Jin, Takashi Hibino

Catalysts Vol. 10 ( 1 ) page： 106 2020.1

Humidity driven transition from insulator to ionic conductor in portland cement Reviewed

Masahiro Nagao, Kazuyo Kobayashi, Tetsuya Hori, Yaorong Li, Takashi Hibino

Materials Vol. 12 ( 22 ) page： 3701 2019.11

Electrolysis of humidified methane to hydrogen and carbon dioxide at low temperatures and voltages Reviewed

Tetsuya Hori, Qiang Ma, Kazuyo Kobayashi, Masahiro Nagao, Shinya Teranishi, Takashi Hibino

International Journal of Hydrogen Energy Vol. 44 ( 5 ) page： 2454 - 2460 2019.1

Intermediate-temperature electrolysis of energy grass Miscanthus sinensis for sustainable hydrogen production Reviewed

Masaya Ito, Tetsuya Hori, Shinya Teranishi, Masahiro Nagao, Takashi Hibino

Scientific Reports Vol. 8 ( 1 ) page： 16186 2018.11

Direct electrolysis of waste newspaper for sustainable hydrogen production: an oxygen-functionalized porous carbon anode Reviewed

Hibino Takashi, Kobayashi Kazuyo, Ito Masaya, Nagao Masahiro, Fukui Mai, Teranishi Shinya

APPLIED CATALYSIS B-ENVIRONMENTAL Vol. 231 page： 191 - 199 2018.9

Language：Japanese Publishing type：Research paper (scientific journal) Publisher：Applied Catalysis B: Environmental

Biomass electrolysis enables hydrogen (H2) production at onset voltages of less than 1 V, depending on the fuel species. However, biofuel derived from biomass not categorized as food and produced from environmentally friendly processes is needed for the development of sustainable strategies. In addition, the biofuel should not require special and expensive procedures for processing. The present report describes the direct electrolysis of waste newspaper for H2 production. Cellulose and lignin included in the newspaper were subject to dissolution and hydrolysis in a phosphoric acid solvent at the anode in a temperature range of 100–175 °C. The resulting decomposition products were electrolyzed to H2 and carbon dioxide (CO2), at low onset voltages (ca. 0.2 V) and high current efficiencies (H2: 1.0, CO2: 0.9). Carbon black functionalized with carbonyl groups showed greater catalytic activity than a Pt/C catalyst for the anode reaction. H2 yield reached ca. 0.2 g per 1 g of newspaper in a batch cell. H2 was produced continuously in a current-density range of 0.15–0.25 A cm−2 while maintaining plateau-like voltage behavior in a flow cell. The energy consumed for electrolysis at a current density of 0.15 A cm−2 was as low as 1.27 kWh (Nm3)−1.

DOI： 10.1016/j.apcatb.2018.03.021

Web of Science

Scopus

Efficient hydrogen production by direct electrolysis of waste biomass at intermediate temperatures Reviewed

Takashi Hibino, Kazuyo Kobayashi, Masaya Ito, Qiang Ma, Masahiro Nagao, Mai Fukui, Shinya Teranishi

ACS Sustainable Chemistry & Engineering Vol. 6 ( 7 ) page： 9360 - 9368 2018.7

Hydrogen production by direct Lignin electrolysis at intermediate temperatures Reviewed

Takashi Hibino, Kazuyo Kobayashi, Masahiro Nagao, Shinya Teranishi,

ChemElectroChem Vol. 4 ( 12 ) page： 3032 - 3036 2017.12

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Papers - HIBINO, Takashi