研究者詳細 - 杉山　貴彦

論文 - 杉山　貴彦

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Numerical Simulation of simulated moving bed chromatography for separation of lithium isotopes 査読有り

Takahiko Sugiyama

Fusion Engineering and Design 200 巻 2024年3月

Hydrogen Isotope (H-2 and D-2) Sorption Study of CHA-Type Zeolites 査読有り

Taguchi Akira, Nakamori Takumi, Yoneyama Yuki, Sugiyama Takahiko, Tanaka Masahiro, Kotoh Kenji, Tachibana Yu, Suzuki Tatsuya

FUSION SCIENCE AND TECHNOLOGY 76 巻 ( 3 ) 頁： 314 - 320 2020年4月

Preparation of Benzo-15-Crown-5 Adsorbents for the Separation of Lithium Isotopes by Displacement Chromatography

Sugiyama Takahiko, Sugiura Kei

FUSION SCIENCE AND TECHNOLOGY 71 巻 ( 4 ) 頁： 473 - 477 2017年5月

Preparation of benzo-15-crown-5 adsorbents for the separation of lithium isotopes by displacement chromatography 査読有り

T. Sugiyama, K. Sugiura

Fusion Science and Technology 71 巻 ( 4 ) 頁： 473-477 2017年

水‐水素化学交換法による水素同位体分離招待有り

杉山貴彦

92 巻 ( 1 ) 頁： 31-38 2016年1月

Separative Analyses of a Chromatographic Column Packed with a Core-shell Adsorbent for Lithium Isotope Separation 査読有り

T. Sugiyama, K. Sugiura, M. Tanaka, Y. Enokida

Fusion Science and Technology 67 巻 ( 3 ) 頁： 584-587 2015年

Longitudinal Dispersion Coefficient Depending on Superficial Velocity of Hydrogen Isotopes Flowing in Column Packed with Zeolite Pellets at 77.4 K 査読有り

K. Kotoh, K. Kubo, S. Takashima, S. Moriyama, M. Tanaka, T. Sugiyama

Fusion Science and Technology 67 巻 ( 2 ) 頁： 439-442 2015年

Dual temperature dual pressure water-hydrogen chemical exchange for water detritiation 査読有り

T. Sugiyama, A. Takada, Y. Morita, K. Kotoh, K. Munakata, A. Taguchi, T. Kawano, M. Tanaka, N. Akata

Fusion Engineering and Design 2015年

Development of a Tritium Monitor Combined with an Electrochemical Tritium Pump Using a Proton Conducting Oxide 査読有り

M. Tanaka, T. Sugiyama

Fusion Science and Technology 67 巻 ( 3 ) 頁： 600-603 2015年

Adsorption Characteristics of Water Vapor on Gear-Pellet and Honeycomb-Pellet Types of Adsorbents Containing A-Type Zeolite 査読有り

A. Nakamura, K. Munakata, K. Hara, S. Narita, T. Sugiyama, K. Kotoh, M. Tanaka, T. Uda

Fusion Science and Technology 67 巻 ( 3 ) 頁： 499-502 2015年

Effect of Air on Energy and Rise-Time Spectra Measured by Proportional Gas Counter 査読有り

T. Kawano, S. Isozumi, Y. Isozumi, M. Tosaki, M. Tanaka, T. Sugiyama

Fusion Science and Technology 67 巻 ( 2 ) 頁： 408-411 2015年

Mathematical models for water vapor absorption on catalyst and adsorbent in atmosphere detritiation and correlation of oxidation rate of hydrogen 査読有り

K. Munakata, K. Hara, T. Sugiyama, M. Tanaka, T. Uda

Fusion Engineering and Design 88 巻 ( 9-10 ) 頁： 2408-2412 2013年

Numerical Simulation of Detritiation System for NIFS with Commercial Catalyst and Adsorbent 査読有り

K. Munakata, K. Hara, T. Sugiyama, K. Kotoh, M. Tanaka, T. Uda

Journal of Plasma and Fusion Research SERIES 10 巻頁： 36-41 2013年

Porosity and water vapor sorption property of new hydrophobic silica beads for CECE catalyst support

A. Taguchi, T. Sugiyama, Y. Morita, M. Tanaka, K. Kotoh, K. Munakata

Annual Report of Hydrogen Isotope Research Center, University of Toyama 33 巻頁： 45-51 2013年

Low-temperature conversion of spent adsorbent to iodine sodalite by a mechanochemical route 査読有り

D. Hirabayashi, Y. Tanada, T. Sugiyama, Y. Enokida, K. Sawada

AICHE Journal 58 巻 ( 8 ) 頁： 2441-2447 2012年

Transient response simulation of gas separation membrane module for an atmosphere detritiation system 査読有り

T. Sugiyama, M. Tanaka, K. Munakata, I. Yamamoto

Fusion Engineering and Design 87 巻頁： 1181-1185 2012年

Lithium isotope separation with displacement chromatography using crown ether resin immobilized on porous silica beads 査読有り

T. Sugiyama, K. Sugiura, M. Tanaka, Y. Enokida

Fusion Engineering and Design 87 巻頁： 1186-1189 2012年

核融合炉実現を目指したトリチウム研究の新展開　5. トリチウムシステム

山西敏彦，波多野雄治，赤丸悟士，朝倉大和，磯部兼嗣，岩井保則，奥野健二，小田卓司，大矢恭久，杉山貴彦，田中知，鳥養祐二，中村博文，林巧，原正憲

88 巻 ( 9 ) 頁： 508-528 2012年

Study on oxidation of hydrogen over commercial catalyst for tritium recovery system 査読有り

K. Hara, K. Munakata, J. Nagane, M. Fukuda, K. Wada, T. Sugiyama, M. Tanaka, T. Uda

Fusion Engineering and Design 87 巻 ( 7-8 ) 頁： 1118-1122 2012年

A simulation model for transient response of a gas separation module using a hollow fiber membrane 査読有り

T. Sugiyama, N. Miyahara, M. Tanaka, K. Munakata, I. Yamamoto

Fusion Engineering and Design 86 巻 ( 9-11 ) 頁： 2743-2746 2011年

Recent activities of R&D on effects of tritium water on confinement materials and tritiated water processing 査読有り

T. Yamanishi, T. Hayashi, Y. Iwai, K. Isobe, M. Hara, T. Sugiyama, K. Okuno

Fusion Engineering and Design 86 巻頁： 2152-2155 2011年

Verification of hydrogen isotope separation by pressure swing adsorption process: Successive volume reduction of isotopic gas mixture using SZ-5A column 査読有り

K. Kotoh, M. Tanaka, S. Takashima, T. Tsuge, Y. Asakura, T. Uda, T. Sugiyama

Fusion Engineering and Design 86 巻頁： 2799-2804 2011年

Successive Volume Reduction of Hydrogen-Isotopic Gaseous Waste by Pressure Swing Adsorption Using SZ-13X Column 査読有り

K. Kotoh, M. Tanaka, T. Tsuge, S. Moriyama, S. Takashima, Y. Asakura, T. Uda, T. Sugiyama

Fusion Science and Technology 60 巻 ( 2 ) 頁： 771-775 2011年

Hydrogen-Tritium Isotope Separation by CECE Process with a Randomly Packed LPCE Column 査読有り

T. Sugiyama, E. Suzuki, M. Tanaka, I. Yamamoto

Fusion Science and Technology 60 巻 ( 4 ) 頁： 1323-1326 2011年

Extraction of Hydrogen and Tritium using High-Temperature Proton Conductor for Tritium Monitoring 査読有り

M. Tanaka, T. Sugiyama, T. Ohshima, I. Yamamoto

Fusion Science and Technology 60 巻 ( 4 ) 頁： 1391-1394 2011年

Successive Hydrogen Isotope Separation/Enrichment by Pressure Swing Adsorption Using 13X Column 査読有り

K. Kotoh, M.Tanaka, T.Tsuge, S. Moriyama, S. Takashima, Y.Asakura, T. Uda, T. Sugiyama

Fusion Science and Technology 60 巻 ( 4 ) 頁： 1355-1358 2011年

Verification of Hydrogen Isotope Separation/Enrichment by Pressure Swing Adsorption Process: Successive Enrichment of Deuterium Using SZ-5A Column 査読有り

K. Kotoh, M. Tanaka, S. Takashima, T. Tsuge, Y. Asakura, T. Uda, T. Sugiyama

Fusion Engineering and Design 85 巻頁： 1992-1998 2010年

Performance Tests of Tritium Separation by LPCE Column at TLK Facility 査読有り

T. Sugiyama, M. Tanaka, I. Cristescu, L. Dörr, S. Welte, R. Michling, Y. Asakura, T. Uda, I. Yamamoto

Fusion Science and Technology 56 巻 ( 2 ) 頁： 861-866 2009年

担当区分：筆頭著者記述言語：英語掲載種別：研究論文（学術雑誌）

The research for the performance improvement of the Liquid Phase Chemical Exchange (LPCE) column has been carried out at Nagoya University in collaboration with National Institute for Fusion Science (NIFS) and Tritium Laboratory Karlsruhe (TLK). Kogel catalysts and Dixon gauze rings were mixed at a certain ratio and packed in the column in a random manner. Performance tests of tritium separation by the column using tritiated water of 26 kBq/cm3 in the electrolyzer were performed at the TLK experimental facility. An effect of axial mixing on the separative performance of the column was examined by a stage-wise model, named Channeling stage model. It was suggested by the analyses that quite a long-distance axial mixing generated in the water phase.

Multi-component Behavior of Hydrogen Isotopes in Zeolite Packed-Beds Used for Cryogenic Pressure Swing Adsorption 査読有り

K. Kotoh, M. Tanaka, T. Sakamoto, S. Takashima, Y. Asakura, T. Uda, T. Sugiyama

Fusion Science and Technology 56 巻 ( 1 ) 頁： 184-189 2009年

Overshooting Breakthrough Curves Formed in Pressure Swing Adsorption Process for Hydrogen Isotope Separation 査読有り

K. Kotoh, M. Tanaka, T. Sakamoto, S. Takashima, Y. Asakura, T. Uda, T. Sugiyama

Fusion Science and Technology 56 巻 ( 1 ) 頁： 173-178 2009年

核融合炉実現を目指したトリチウム研究の新展開　6. トリチウムの閉じ込めに関わる高濃度トリチウム水および有機物の化学的現象の解明

山西敏彦，岩井保則，磯部兼嗣，杉山貴彦

85 巻 ( 10 ) 頁： 716-725 2009年

Hydrogen Isotope Separation by Combined Electrolysis and Random-packed Chemical Exchange Column

T. Sugiyama, I. Yamamoto

2nd Japan-China Workshop on Blanket and Tritium Technology 頁： 92-95 2008年5月

Development of an improved LPCE column for the TLK facility with the help of the channeling stage model 査読有り

T. Sugiyama, M. Tanaka, K. Munakata, Y. Asakura, T. Uda, I. Yamamoto, I. Cristescu, L. Doerr

Fusion Engineering and Design 83 巻頁： 1442-1446 2008年

担当区分：筆頭著者記述言語：英語掲載種別：研究論文（学術雑誌）

The research for the performance improvement of the Liquid Phase Chemical Exchange (LPCE) column has been carried out at Nagoya University with the collaboration of National Institute for Fusion Science (NIFS) and Tritium Laboratory Karlsruhe (TLK). Kogel catalysts and Dixon gauze rings were mixed at a certain ratio and packed in the column homogeneously. A stage-wise model, named Channeling stage model, was also developed to predict separative performances of the column. In order to design a LPCE column to be tested at the TLK experimental facility we examined the effect of the catalyst packed ratio and the gas-liquid ratio on the separative performance of the column. The optimal value of the catalyst packed ratio was obtained to 30 %. The specifications of the column and the operating conditions of the equipment were reported.

The background levels of atmospheric tritium concentration in the environment at NIFS Toki site of Japan 査読有り

T. Uda, M. Tanaka, T. Sugiyama, T. Yamaguchi, N. Momoshima

Fusion Science and Technology 54 巻 ( 1 ) 頁： 281-284 2008年

Experimental verification of hydrogen isotope separation by pressure swing adsorption 査読有り

K. Kotoh, M. Tanaka, Y. Nakamura, T. Sakamoto, Y. Asakura, T. Uda, T. Sugiyama

Fusion Science and Technology 54 巻 ( 2 ) 頁： 411-414 2008年

Breakthrough curve analysis of pressure swing adsorption for hydrogen isotope separation 査読有り

K. Kotoh, M. Tanaka, T. Sakamoto, Y. Nakamura, Y. Asakura, T. Uda, T. Sugiyama

Fusion Science and Technology 54 巻 ( 2 ) 頁： 415-418 2008年

Effects of the gas-liquid ratio on the optimum catalyst quantity for the CECE process with a homogeneously packed LPCE column 査読有り

T. Sugiyama, A. Ushida, I. Yamamoto

Fusion Engineering and Design 83 巻頁： 1447-1450 2008年

担当区分：筆頭著者記述言語：英語掲載種別：研究論文（学術雑誌）

The effect of the gas-liquid ratio (G/L) on the optimal quantity of the catalyst was studied experimentally in a homogeneously packed bed used for a Combined Electrolysis Catalytic Exchange (CECE) process for hydrogen isotope separation. When the value of G/L was 1.7 total separation factors were relatively small and the optimal quantity of the catalyst could not be found. On the other hand, when the values of G/L were 0.9 and 0.7 the values of total separation factors have maximums and the optimal quantities of the catalyst were clearly obtained.

核融合炉トリチウム水処理システムの研究開発動向

山西敏彦，岩井保則，磯部兼嗣，杉山貴彦

プラズマ・核融合学会誌 83 巻 ( 6 ) 頁： 545-559 2007年6月

記述言語：日本語

核融合炉施設は核融合を起こす燃料として，放射性物質であるトリチウムガスおよび副次的に生じる高濃度トリチウム水を大量に取り扱う施設であり，施設内に設ける燃料循環システムにて処理を行い，燃料サイクルを施設内に閉じてしまうことが必要となる。したがって，核融合炉の安全確保と燃料サイクルの確立を目指す上で，トリチウム水の処理は鍵となる技術である。本報では，ITERにおけるトリチウム水処理システムの開発経緯，第一壁冷却水やブランケット冷却水の処理までを見通した核融合原型炉に向けた水処理総合システムの研究開発状況を紹介する。

Present Status of Hydrogen Isotope Separation by CECE Process at the NIFS 査読有り

T. Sugiyama, Y. Asakura, T. Uda, T. Shiozaki, Y. Enokida, I. Yamamoto

Fusion Engineering and Design 81 巻頁： 833-838 2006年

担当区分：筆頭著者記述言語：英語掲載種別：研究論文（学術雑誌）

Isotope separation experiments of hydrogen and deuterium are performed with two types of packed beds filled with Kogel catalysts (4.0-6.7 mm spherical, 0.8 wt% Pt deposited) and Dixon gauze rings (6 mm outer diameter, 6 mm height). One is the layered bed where layers of Kogel catalysts and that of Dixon gauze rings are filled in the column alternately. The other is the homogeneous bed where Kogel catalysts and Dixon gauze rings are mixed and filled in the column homogeneously. The separative performance of the homogeneous bed is appreciably greater than that of the layered bed, where the quantities of the catalysts are equal for both beds.

Developments of gaseous water, hydrogen and methane sampling system for environmental tritium monitoring 査読有り

T. Uda, T. Sugiyama, M. Tanaka, K. Munakata, N. Momoshima

Fusion Engineering and Design 81 巻頁： 1385-1390 2006年

Measurement of Breakthrough Curves on Pressure Swing Adsorption for Hydrogen Isotope Separation 査読有り

T. Sugiyama, Y. Asakura, T. Uda, K. Kotoh

Fusion Science and Technology 48 巻 ( 1 ) 頁： 163-166 2005年

Hydrogen Isotope Separation by Combined Electrolysis Catalytic Exchange under Reduced Pressure 査読有り

T. Sugiyama, Y. Asakura, T. Uda, Y. Abe, T. Shiozaki, Y. Enokida, I. Yamamoto

Fusion Science and Technology 48 巻 ( 1 ) 頁： 132-135 2005年

Application of New Technologies for Gaseous Tritium Recovery and Monitoring 査読有り

Y. Asakura, T. Sugiyama, T. Kawano, T. Uda, M. Tanaka, N. Tsuji, K. Katahira, H. Iwahara

Fusion Science and Technology 48 巻 ( 1 ) 頁： 401-404 2005年

Development of a High Performance Catalyst for Oxidation of Tritiated Hydrogen and Methane Gases 査読有り

T. Uda, T. Sugiyama, Y. Asakura, K. Munakata, M. Tanaka

Fusion Science and Technology 48 巻 ( 1 ) 頁： 480-483 2005年

Preliminary Experiments on Hydrogen Isotope Separation by Water-Hydrogen Chemical Exchange under Reduced Pressure 査読有り

T. Sugiyama, Y. Asakura, T. Uda, Y. Abe, T. Shiozaki, Y. Enokida , I. Yamamoto

Journal of Nuclear Science and Technology 41 巻 ( 6 ) 頁： 696-701 2004年6月

Application of Proton-conducting Ceramics and Polymer Permeable Membranes for Gaseous Tritium Recovery 査読有り

Y. Asakura, T. Sugiyama, T. Kawano, T. Uda, M. Tanaka, N. Tsuji, K. Katahira, H. Iwahara

Journal of Nuclear Science and Technology 41 巻 ( 10 ) 頁： 863-870 2004年

Stability Test and Improvement of Hydrogen Analyzer with Trace Reduction Detector 査読有り

T. Kawano, N. Tsuboi, H. Tsujii, T. Sugiyama, Y. Asakura, T. Uda

Journal of Chromatography A 1023 巻頁： 123-127 2004年

Trace Analysis of Deuterium by Reduction of Mercury (II) Oxide 査読有り

T. Kawano, N. Tsuboi, H. Tsujii, T. Sugiyama, Y. Asakura, T. Uda

Radioisotopes 53 巻 ( 1 ) 頁： 27-32 2004年

Infinitesimal Concentration Hydrogen Analyzer using Trace Reduction Detector (TRD) 査読有り

T. Kawano, N. Tsuboi, H. Tsujii, T. Sugiyama, Y. Asakura, T. Uda

Japan Journal of Applied Physics 42 巻頁： L549-L551 2003年

Separative Analyses of Packed Water Distillation Column with Channeling Stage Model 査読有り

T. Sugiyama, Y. Enokida, I. Yamamoto

Journal of Nuclear Science and Technology 37 巻 ( 3 ) 頁： 273-280 2000年3月

A Solution of a Material Balance Equation of Channeling Stage Model for a Simple Case of a Water Distillation Column 査読有り

T. Sugiyama, Y. Enokida, I. Yamamoto

Journal of Nuclear Science and Technology 36 巻 ( 10 ) 頁： 959-961 1999年10月

Effect of Partition Wall within Packings on Separative Performances of Water Distillation for H2O-HTO Isotope Separation 査読有り

T. Sugiyama, Y. Enokida, I. Yamamoto

Journal of Nuclear Science and Technology 36 巻 ( 8 ) 頁： 691-697 1999年8月

Effects of partition wall within packings on separative performances of water distillation for H2O-HTO isotope separation

Sugiyama T, Enokida Y, Yamamoto I

JOURNAL OF NUCLEAR SCIENCE AND TECHNOLOGY 36 巻 ( 8 ) 頁： 691 - 697 1999年8月

Effect of Inner Radius of Wetted-wall Column on Separative Performance of H2O-HTO Water Distillation 査読有り

T. Sugiyama, Y. Enokida, I. Yamamoto

Journal of Nuclear Science and Technology 35 巻 ( 10 ) 頁： 723-727 1998年10月

Effect of inner radius of wetted-wall column on separative performance of H<sub>2</sub>O-HTO water distillation

Sugiyama, T; Enokida, Y; Yamamoto, I

JOURNAL OF NUCLEAR SCIENCE AND TECHNOLOGY 35 巻 ( 10 ) 頁： 723 - 727 1998年10月

出版者・発行元：Journal of Nuclear Science and Technology

Developing a computer code which solves concentration profiles simultaneously for vapor and liquid phases, we analyzed an effect of inner radius of wetted-wall column on separative performances of water distillation for H2O-HTO isotope separation. Results through the code were compared with experiments for H2O-HTO wetted-wall water distillation under the total reflux condition with columns of 3 and 8 mm of inner radius R. Total separation factors of R=3mm were larger than those of R=8mm, and the fact was well predicted by a numerical analysis. The total separation factors for theoretically maximum vaporization rate constant kv, A=1.57 × 104 cm/s gave a virtual its upper limit in the range of relatively large Reynolds number. © 1998 Taylor & Francis Group, LLC.

DOI： 10.1080/18811248.1998.9733933

Web of Science

Scopus

Simultaneous Solution of Concentration Profiles in Vapor-liquid Phases of Wetted-wall Distillation Column for H2O-HTO Isotope Separation 査読有り

T. Sugiyama, Y. Kato, Y. Enokida, I. Yamamoto

Journal of Nuclear Science and Technology 35 巻 ( 1 ) 頁： 60-65 1998年1月

Simultaneous solution of concentration profiles in vapor-liquid phases of wetted-wall distillation column for H<sub>2</sub>O-HTO isotope separation

Sugiyama, T; Kato, Y; Enokida, Y; Yamamoto, I

JOURNAL OF NUCLEAR SCIENCE AND TECHNOLOGY 35 巻 ( 1 ) 頁： 60 - 65 1998年1月

出版者・発行元：Journal of Nuclear Science and Technology

A simulation model was proposed for prediction of H2O-HTO separative performances of water distillation by a wetted-wall column. A wetted-wall column was assumed to be a circular tube, and mole-fraction profiles in the tube were obtained by coupling the equations which describe diffusion processes of both vapor and liquid phases and by solving the equations simultaneously. It was found that the calculations for constant mole-fraction boundary with high mass-transfer rate resulted in overestimations of degree of separation. The relative difference of the HETP value for constant mole-fraction boundary from that for the present model was −19% when P = 101.3kPa, T = 373K, R = 0.8 cm, H = 100 cm, k v, A = 1.0 × 104 cm/s and Rev = 660. © 1998 Taylor and Francis Group, LTD.

DOI： 10.1080/18811248.1998.9733820

Web of Science

Scopus

Channeling Stage Model for Separative Analysis of Packed Water Distillation Column 査読有り

T. Sugiyama, Y. Kamewaka, Y. Enokida, I. Yamamoto

Fusion Engineering and Design 39-40 巻頁： 1027-1032 1998年

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